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Suitability of common models to estimate hydrology and diffuse water pollution in North-eastern German lowland catchments with intensive agricultural land use

Muhammad WASEEM, Frauke KACHHOLZ, Jens TRÄNCKNER

《农业科学与工程前沿（英文）》 2018年第5卷第4期页码 420-431 doi: 10.15302/J-FASE-2018243

摘要：

Various process-based models are extensively being used to analyze and forecast catchment hydrology and water quality. However, it is always important to select the appropriate hydrological and water quality modeling tools to predict and analyze the watershed and also consider their strengths and weaknesses. Different factors such as data availability, hydrological, hydraulic, and water quality processes and their desired level of complexity are crucial for selecting a plausible modeling tool. This review is focused on suitable model selection with a focus on desired hydrological, hydraulic and water quality processes (nitrogen fate and transport in surface, subsurface and groundwater bodies) by keeping in view the typical lowland catchments with intensive agricultural land use, higher groundwater tables, and decreased retention times due to the provision of artificial drainage. In this study, four different physically based, partially and fully distributed integrated water modeling tools, SWAT (soil and water assessment tool), SWIM (soil and water integrated model), HSPF (hydrological simulation program– FORTRAN) and a combination of tools from DHI (MIKE SHE coupled with MIKE 11 and ECO Lab), have been reviewed particularly for the Tollense River catchment located in North-eastern Germany. DHI combined tools and SWAT were more suitable for simulating the desired hydrological processes, but in the case of river hydraulics and water quality, the DHI family of tools has an edge due to their integrated coupling between MIKE SHE, MIKE 11 and ECO Lab. In case of SWAT, it needs to be coupled with another tool to model the hydraulics in the Tollense River as SWAT does not include backwater effects and provision of control structures. However, both SWAT and DHI tools are more data demanding in comparison to SWIM and HSPF. For studying nitrogen fate and transport in unsaturated, saturated, and river zone, HSPF was a better model to simulate the desired nitrogen transformation and transport processes. However, for nitrogen dynamics and transformations in shallow streams, ECO Lab had an edge due its flexibility for inclusion of user-desired water quality parameters and processes. In the case of SWIM, most of the input data and governing equations are similar to SWAT but it does not include water bodies (ponds and lakes), wetlands and drainage systems. In this review, only the processes that were needed to simulate the Tollense River catchment were considered, however the resulted model selection criteria can be generalized to other lowland catchments in Australia, North-western Europe and North America with similar complexity.

关键词： diffuse pollution ECO Lab HSPF lowland catchment MIKE 11 MIKE SHE modeling tools SWAT SWIM Tollense River water quality

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Palmitoylation of GNAQ/11 is critical for tumor cell proliferation and survival in GNAQ/11-mutant uveal

《医学前沿（英文）》 2022年第16卷第5期页码 784-798 doi: 10.1007/s11684-021-0911-0

摘要： More than 85% of patients with uveal melanoma (UM) carry a GNAQ or GNA11 mutation at a hotspot codon (Q209) that encodes G protein α subunit q/11 polypeptides (Gα_q/11). GNAQ/11 relies on palmitoylation for membrane association and signal transduction. Despite the palmitoylation of GNAQ/11 was discovered long before, its implication in UM remains unclear. Here, results of palmitoylation-targeted mutagenesis and chemical interference approaches revealed that the loss of GNAQ/11 palmitoylation substantially affected tumor cell proliferation and survival in UM cells. Palmitoylation inhibition through the mutation of palmitoylation sites suppressed GNAQ/11^Q209L-induced malignant transformation in NIH3T3 cells. Importantly, the palmitoylation-deficient oncogenic GNAQ/11 failed to rescue the cell death initiated by the knock down of endogenous GNAQ/11 oncogenes in UM cells, which are much more dependent on Gα_q/11 signaling for cell survival and proliferation than other melanoma cells without GNAQ/11 mutations. Furthermore, the palmitoylation inhibitor, 2-bromopalmitate, also specifically disrupted Gα_q/11 downstream signaling by interfering with the MAPK pathway and BCL2 survival pathway in GNAQ/11-mutant UM cells and showed a notable synergistic effect when applied in combination with the BCL2 inhibitor, ABT-199, in vitro. The findings validate that GNAQ/11 palmitoylation plays a critical role in UM and may serve as a promising therapeutic target for GNAQ/11-driven UM.

关键词： uveal melanoma mutant GNAQ/11 palmitoylation BCL2 combination target therapy

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Effects of the SAPO-11 synthetic process on dehydration of ethanol to ethylene

Lina WU, Xiaoxing SHI, Qun CUI, Haiyan WANG, He HUANG

《化学科学与工程前沿（英文）》 2011年第5卷第1期页码 60-66 doi: 10.1007/s11705-010-0540-7

摘要： The effects of the synthetic condition of SAPO-11 molecular sieves on ethanol dehydration to ethylene were studied. Product-compositions, ethanol conversion, and selectivity to ethylene of synthesized and commercial SAPO-11 molecular sieves were compared. Results are as follows: the optimal synthetic conditions for SAPO-11 molecular sieves are adding pseudoboehmite before orthophoshporic, using di-n- propylamine as the template, having a mass fraction of 40% colloidal silica as the silica source and the starting gel obtained, and running at 200°C for 48 h. From the patterns of NH -TPD, the amount of acid synthesized by SAPO-11 molecular sieves is less than that by commercial SAPO-11 molecular sieves, and has a stronger weak acid. Also, ethanol conversion and selectivity to ethylene reached 99% at 280°C on synthesized SAPO-11, lower by 20°C compared to commercial SAPO-11. For two SAPO-11 molecular sieves, the by-products in the gas phase are mainly ethane, propane, propene, isobutane, n-butane, propadiene, butylene and some higher hydrocarbons. The by-products in the liquid phase are ethyl ether and acetaldehyde.

关键词： SAPO-11 molecular sieves synthesis ethanol ethylene dehydration

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Retraction note to: Industrial bio-based plant aggregates as hygric and insulating construction materials for energy efficient building

Yunhong Jiang, Mike Lawrence, Meng Zhang, Jiandong Cui

《化学科学与工程前沿（英文）》 doi: 10.1007/s11705-021-2039-9

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Mechanistic insights into the selective photocatalytic degradation of dyes over TiO/ZSM-11

《环境科学与工程前沿（英文）》 2023年第17卷第8期 doi: 10.1007/s11783-023-1701-5

摘要：

● TiO₂/ZSM-11 was prepared by a facile solid state dispersion method.

关键词： Selective dye degradation Photocatalysis TiO₂ ZSM-11 Chemisorption

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Organic Contaminants in Chinese Surface Water: Identification of Priority Pollutants” [Engineering 11 Corrigendum

Mengmeng Zhong, Tielong Wang, Wenxing Zhao, Jun Huang, Bin Wang, Lee Blaney, Qingwei Bu, Gang Yu

《工程（英文）》 2023年第31卷第12期页码 139-140 doi: 10.1016/j.eng.2022.09.001

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China’s Sponge City construction: A discussion on technical approaches

Haifeng Jia, Zheng Wang, Xiaoyue Zhen, Mike Clar, Shaw L. Yu

《环境科学与工程前沿（英文）》 2017年第11卷第4期 doi: 10.1007/s11783-017-0984-9

摘要： Since 2014, China has been implementing the Sponge City Construction initiative, which represents an enormous and unprecedented effort by any government in the world for achieving urban sustainability. According to preliminary estimates, the total investment on the Sponge City Plan is roughly 100 to 150 million Yuan (RMB) ($15 to $22.5 million) average per square kilometer or 10 Trillion Yuan (RMB) ($1.5 Trillion) for the 657 cities nationwide. The Sponge City Plan (SCP) calls for the use of natural processes such as soil and vegetation as part of the urban runoff control strategy, which is similar to that of low impact development (LID) and green infrastructure (GI) practices being promoted in many parts of the world. The SCP includes as its goals not only effective urban flood control, but also rainwater harvest, water quality improvement and ecological restoration. So far, the SCP implementation has encountered some barriers and challenges due to many factors. The present paper presents a review of those barriers and challenges, offers discussions and recommendations on several technical aspects such as control goals and objectives; planning/design and construction of LID/GI practices; performance evaluation. Several key recommendations are proposed on Sponge City implementation strategy, Site-specific regulatory framework and technical guidance, Product innovation and certification, LID/GI Project financing, LID/GI professional training and certification, public outreach and education. It is expected that the successful implementation of the SCP not only will bring about a sustainable, eco-friendly urbanization process in China, but also contribute enormously to the LID/GI research and development with the vast amount of relevant data and experiences generated from the Sponge City construction projects.

关键词： Low impact development (LID) Green infrastructure (GI) Sponge City Barriers Construction strategies

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Industrial bio-based plant aggregates as hygric and insulating construction materials for energy efficient building

Yunhong Jiang, Mike Lawrence, Meng Zhang, Jiandong Cui

《化学科学与工程前沿（英文）》 2022年第16卷第10期页码 1532-1532 doi: 10.1007/s11705-020-1960-7

摘要： In this paper, the bulk density, microstructure, porosity and pore size distribution of the selected aggregates, including hemp shiv, flax shiv, rape shiv and wheat straw, are fully studied due to these properties are highly related to their excellent characteristics and more or less linked to the properties of the final product. The scanning electron microscope results showed all the selected aggregates have a highly porous and complex hierarchical structure, whereas the arrangement of pores and the thickness of cell wall are significantly different among these aggregates. All the selected aggregates had a low bulk density ranging from 30 to 130 kg∙m and a high porosity between 75.81% and 88.74%. The thermal conductivity of the selected bio-aggregates ranged from 0.04 to 0.06 W∙m ∙K . The thermal conductivity of the selected aggregates was not only depending on the bulk density of the sample but also depending on the raw material. Hemp shiv, rape shiv and flax shiv were excellent hygric regulators with moisture buffer value ( ) ranging from 2.07 to 2.36 g∙m ∙%RH , whereas, wheat straw had a lower MBV value ranging from 1.76 to 1.97 g∙m ∙%RH . The results showed that particle size does not affect the value. The value increases linearly with bulk density.

关键词： bio-based aggregates density porosity thermal conductivity hygric properties

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Dynamic mechanism for the decline of China’s energy intensity during the 11th FYP (Five-Year Plan)

Minghui LI

《能源前沿（英文）》 2011年第5卷第3期页码 237-249 doi: 10.1007/s11708-010-0130-x

摘要： From 2006 to 2009, the aggregate energy intensity of China fell by 14.38%, which means that China has made substantial progress towards its goal of achieving approximately a 20% reduction in energy intensity during the period of the 11th FYP (Five-Year Plan). This paper describes some new properties of the mechanism for the decrease in China’s energy intensity since the beginning of the 11th FYP. First, compared with the period of the 10th FYP, technical, structural, and residential energy-savings have been improved to a certain extent. Secondly, unlike the dynamic mechanism before 2000, technical energy savings have been the main driver of momentum since the beginning of the 11th FYP. Next, although structural energy savings are not the main factor, they are still a key factor for the decrease in energy intensity. Finally, residential energy savings are still a stable driver of momentum for the decline in China’s energy intensity.

关键词： energy intensity structural energy savings technical energy savings

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齐岳山隧道F11高压富水断层带注浆施工技术

卓越,孙国庆

《中国工程科学》 2009年第11卷第12期页码 82-86

摘要：目前正在施工的齐岳山隧道F11断层破碎带，水压高、水量大、地质条件复杂，成为唯一制约全线的主要技术难题。以平导F11断层的注浆施工治水防坍为实例，介绍F11高水压断裂带治水防坍新方案、新工艺及效果检查新方法等，为以后类似工程积累经验。

关键词：齐岳山隧道断层破碎带技术难题新方案新工艺效果检查

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WLAN 802.11/11b数据加密机制的安全分析

宋宇波,胡爱群,蔡天佑

《中国工程科学》 2004年第6卷第10期页码 32-38

摘要：

在802.11标准中的加密采用WEP协议，用于提供链路层数据传输的安全保护。目前，在原有EP的基础上提出了一些改进方案，能提高WEP的安全性能，但理论上缺少严密的安全分析。笔者通过数学模型对这些解决方案以及原有WEP协议进行量化分析，推导出机制内各模块与整个安全机制间安全性能的对应函数关系，并比较了这些方案间安全性能的差异，证明这些安全机制可以提高原有WEP的安全性能，在理论上为用户提供如何构造满足所需安全性能的WLAN数据加密增强机制。

关键词： WLAN 安全分析 WEP 密钥更新

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DyFe₁₁Ti磁结构及其自旋重取向的中子衍射研究 Article

Olivier Isnard, Eder J. Kinast

《工程（英文）》 2020年第6卷第2期页码 153-157 doi: 10.1016/j.eng.2019.11.009

摘要：

本文报道了通过中子粉末衍射探测DyFe₁₁Ti的磁结构及其热演化规律。使用了变温中子衍射技术来测量磁矩及其取向的温度依赖性。

关键词：中子衍射，磁相图，晶体结构

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Planetary Homeostasis of Reactive Nitrogen Through Anaerobic Ammonium Oxidation

Callbeck,Shanyun Wang,Liping Jiang,Asheesh Kumar Yadav,Jan Vymazal,Mike S. M.

《工程（英文）》 doi: 10.1016/j.eng.2023.09.013

摘要： The availability of nitrogen (N) is crucial for both the productivity of terrestrial and aquatic ecosystems globally. However, the overuse of artificial fertilizers and the energy required to fix nitrogen have pushed the global nitrogen cycle (N-cycle) past its safe operating limits, leading to severe nitrogen pollution and the production of significant amounts of greenhouse gas nitrous oxide (N2O). The anaerobic ammonium oxidation (anammox) mechanism can counteract the release of ammonium and N2O in many oxygen-limited situations, assisting in the restoration of the homeostasis of the Earth’s N biogeochemistry. In this work, we looked into the characteristics of the anammox hotspots’ distribution across various types of ecosystems worldwide. Anammox hotspots are present at diverse oxic–anoxic interfaces in terrestrial systems, and they are most prevalent at the oxic–anoxic transition zone in aquatic ecosystems. Based on the discovery of an anammox hotspot capable of oxidizing ammonium anoxically into N2 without N2O by-product, we then designed an innovative concept and technical routes of nature-based anammox hotspot geoengineering for climate change, biodiversity loss, and efficient utilization of water resources. After 15 years of actual use, anammox hotspot geoengineering has proven to be effective in ensuring clean drinking water, regulating the climate, fostering plant and animal diversity, and enhancing long-term environmental quality. The sustainable biogeoengineering of anammox could be a workable natural remedy to resolve the conflicts between environmental pollution and food security connected to N management.

关键词： biogeochemical N-cycle oxic–anoxic interface nature-based solution biogeoengineering nitrogen sustainable development

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PRODUCTION OF NEW WAP-8294A CYCLODEPSIPEPTIDES BY THE BIOLOGICAL CONTROL AGENT LYSOBACTER ENZYMOGENES OH11

《农业科学与工程前沿（英文）》 2022年第9卷第1期页码 120-132 doi: 10.15302/J-FASE-2021410

摘要：

Naturally-occurring environmental microorganisms may provide ‘green’ and effective biocontrol tools for disease management in agricultural crops. Due to the constant threat of resistant pathogens there is a pressing and continual need to search for new biocontrol tools. This study investigated the production of new analogs of WAP-8294A compounds by the biocontrol agent Lysobacter enzymogenes OH11 through biosynthetic engineering. WAP-8294As are a family of natural cyclic lipodepsipeptides with potent activity against Gram-positive bacteria. A series of genetic manipulations was therefore conducted on the accessory genes in the WAP biosynthetic gene cluster. The resulting strains containing a single-point mutation in ORF4, which was predicted to encode a 2-ketoglutarate dependent dioxygenase, produced deoxy-WAP-8294As. This result provides evidence for the function of ORF4 in catalyzing β-hydroxylation of the D-asparagine residue in WAP-8294As. In addition, six new analogs of WAP-8294As were identified by UHPLC-HR-MS/MS. This is the first attempt to produce new WAP-8294As in Lysobacter and shows that the spectrum of the biocontrol compounds may be expanded through the manipulation of biosynthetic genes.

关键词： biocontrol / biosynthesis / Lysobacter / natural products / WAP-8294A

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Co-conversion of methanol and

Shumei Wei, Yarong Xu, Zhaoyang Jin, Xuedong Zhu

《化学科学与工程前沿（英文）》 2020年第14卷第5期页码 783-792 doi: 10.1007/s11705-019-1868-2

摘要： The conversion of -hexane and methanol into value-added aromatic compounds is a promising method for their industrially relevant utilization. In this study, intergrown ZSM-5/ZSM-11 crystals were synthesized and their resulting catalytic performance was investigated and compared to those of the isolated ZSM-5 and ZSM-11 zeolites. The physicochemical properties of ZSM-5/ZSM-11 intergrown zeolite were analyzed using X-ray diffraction, N isothermal adsorption-desorption, the temperature-programmed desorption of ammonium, scanning electron microscopy, Fourier transform infrared spectra of adsorbed pyridine, and nuclear magnetic resonance of Al , and compared with those of the ZSM-5 and ZSM-11 zeolites. The catalytic performances of the materials were evaluated during the co-feeding reaction of methanol and -hexane under the fixed bed conditions of 400°C, 0.5 MPa (N ), methanol꞉ -hexane= 7꞉3 (mass ratio), and weight hourly space velocity= 1 h (methanol). Compared to the ZSM-5 and ZSM-11 zeolites, the ZSM-5/ZSM-11 zeolite exhibited the largest specific surface area, a unique crystal structure, moderate acidity, and suitable Brønsted/Lewis acid ratio. The evaluation results showed that ZSM-5/ZSM-11 catalyst exhibited better catalytic reactivity than the ZSM-5 and ZSM-11 catalysts in terms of methanol conversion rate, -hexane conversion rate, and aromatic selectivity. The outstanding catalytic property of the intergrown ZSM-5/ZSM-11 was attributed to the enhanced diffusion associated with its unique crystal structure. The benefit of using zeolite intergrowth in the co-conversion of methanol and alkanes offers a novel route for future catalyst development.

关键词： ZSM-5/ZSM-11 methanol n-hexane cofeeding aromatics

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标题作者时间类型操作

Suitability of common models to estimate hydrology and diffuse water pollution in North-eastern German lowland catchments with intensive agricultural land use

Muhammad WASEEM, Frauke KACHHOLZ, Jens TRÄNCKNER

期刊论文

Palmitoylation of GNAQ/11 is critical for tumor cell proliferation and survival in GNAQ/11-mutant uveal

期刊论文

Effects of the SAPO-11 synthetic process on dehydration of ethanol to ethylene

Lina WU, Xiaoxing SHI, Qun CUI, Haiyan WANG, He HUANG

期刊论文

Retraction note to: Industrial bio-based plant aggregates as hygric and insulating construction materials for energy efficient building

Yunhong Jiang, Mike Lawrence, Meng Zhang, Jiandong Cui

期刊论文

Mechanistic insights into the selective photocatalytic degradation of dyes over TiO/ZSM-11

期刊论文